Reviews and Special Topics

Research progress of graphene and derived oil removal materials

  • Chi Su ,
  • Chenglei Zhang
Expand
  • 1. CNOOC Energy Technology & Services Limited,Beijing 100027,China
    2. Hebei University of Technology

Received date: 2021-03-15

  Online published: 2021-07-13

Abstract

The recovery process of crude oil or offshore oil leakage will produce a large amount of oily sewage,which brings great threat to the environment.Graphene and derived materials have large specific surface area,special pore structure and so on,which have attracted wide attention in the field of oil removal from oil-containing wastewater.The research progress of graphene-derived oil removal materials such as 3D graphene and graphene composite membrane in the treatment of oily waste was reviewed.The research on 3D graphene oil-absorbing materials was aimed to optimize the micropore structure,surface wettability,and improve the mechanical properties and service life.And the oil-water separation materials of graphene composite membrane mainly improved the flux,antifouling ability and stability of the membrane.At present,the synthesis process of graphene and derived oil removal materials was complicated and the stability was poor.In the future,the research on graphene and derived deoiling materials wouldl focus on reducing cost,improving stability and applicability.

Cite this article

Chi Su , Chenglei Zhang . Research progress of graphene and derived oil removal materials[J]. Inorganic Chemicals Industry, 2021 , 53(7) : 30 -35 . DOI: 10.19964/j.issn.1006-4990.2021-0148

References

[1] Chen P, Yin D, Song P, et al. Demulsification and oil recovery from oil-in-water cutting fluid wastewater using electrochemical micromembrane technology[J]. Journal of Cleaner Production, 2020, 244(13):1-8.
[2] 李威, 任瑞鹏. 石墨烯基吸油材料的研究进展[J]. 现代化工, 2017, 37(8):19-22,24.
[3] Tran V T, Xu X, Mredha M T I, et al. Hydrogel bowls for cleaning oil spills on water[J]. Water Research, 2018, 145:640-649.
[4] Gupta R K, Dunderdale G J, England M W, et al. Oil/water separa-tion techniques:A review of recent progresses and future directio-ns[J]. Journal of Materials Chemistry A, 2017, 5(31):16025-16058.
[5] 刘娟, 赵亚溥, 胡斌, 等. 油水乳状液的稳定机理及其化学破乳技术的研究进展[J]. 化工进展, 2013, 32(4):891-897.
[6] 杨玉洁, 陈雯雯, 张倩, 等. 聚结技术及其乳化油水分离性能[J]. 化工进展, 2019, 38(z1):10-18.
[7] Ni Long, Tian Jinyi, Song Tao, et al. Optimizing geometric parame-ters in hydrocyclones for enhanced separations:A review and persp-ective[J]. Separation & Purification Reviews, 2019, 48(1):30-51.
[8] Krebsz M, Pasinszki T, Tung T T, et al. Multiple applications of bio-graphene foam for efficient chromate ion removal and oil-water sep-aration[J]. Chemosphere, 2021, 263:1-12.
[9] Meng L, Sun Y, Gong H, et al. Research progress of the application of graphene-based materials in the treatment of water pollutants[J]. Carbon, 2019, 153:804-806.
[10] Qin L, Liu W F, Liu X G, et al. A review of nano-carbon based molecularly imprinted polymer adsorbents and their adsorption mechanism[J]. New Carbon Materials, 2020, 35(5):459-485.
[11] Wang Y, Wang B, Wang J, et al. Superhydrophobic and superoleo-philic porous reduced graphene oxide/polycarbonate monoliths for high-efficiency oil/water separation[J]. Journal of Hazardous Materials, 2018, 344:849-856.
[12] Zhou S, Zhou X, Hao G, et al. Property control of graphene aerogels by in situ growth of silicone polymer[J]. Applied Surface Science, 2018, 439:946-953.
[13] 刁帅, 刘会娥, 陈爽, 等. 软模板法石墨烯气凝胶的可控制备及其吸油性能[J]. 化工进展, 2020, 39(7):2742-2750.
[14] Liu Y, Zhang Y, Liu Y, et al. Super heating/cooling rate enabled by microwave shock on polymeric graphene foam for high performa-nce lithium-sulfur batteries[J]. Carbon, 2021, 173:809-816.
[15] Lu Z, Xu X, Chen Y, et al. Nitrogen and sulfur co-doped grapheme aerogel with hierarchically porous structure for high-performance supercapacitors[J]. Green Energy & Environment, 2020, 5(1):69-75.
[16] Xu L, Xiao G, Chen C, et al. Superhydrophobic and superoleophilic graphene aerogel prepared by facile chemical reduction[J]. Journal of Materials Chemistry A, 2015, 3(14):7498-7504.
[17] Maleki H. Recent advances in aerogels for environmental remedia-tion applications:A review[J]. The Chemical Engineering Journal, 2016, 300:98-118.
[18] Wang S, Wang X, Shi X Y, et al. A three-dimensional polyoxomet-alate/graphene aerogel as a highly efficient and recyclable absor-bent for oil/water separation[J]. New Carbon Materials, 2021, 36(1):189-197.
[19] Chi C, Xu H, Zhang K, et al. 3D hierarchical porous graphene aero-gels for highly improved adsorption and recycled capacity[J]. Ma-terials Science and Engineering:B, 2015, 194:62-67.
[20] Chen C, Li F, Zhang Y, et al. Compressive,ultralight and fire-resi-stant lignin-modified graphene aerogels as recyclable absorbents for oil and organic solvents[J]. Chemical Engineering Journal, 2018, 350:173-180.
[21] Zhang S, Liu G, Gao Y, et al. A facile approach to ultralight and recyclable 3D self-assembled copolymer/graphene aerogels for ef-ficient oil/water separation[J]. Science of the Total Environment, 2019, 694:1-11.
[22] Mi H, Jing X, Xie H, et al. Magnetically driven superhydrophobic silica sponge decorated with hierarchical cobalt nanoparticles for selective oil absorption and oil/water separation[J]. Chemical Engineering Journal, 2018, 337:541-551.
[23] Chen B, Ma Q, Tan C, et al. Carbon-based sorbents with three-di-mensional architectures for water remediation[J]. Small, 2015, 11(27):3319-3336.
[24] Kabiri S, Tran D N H, Altalhi T, et al. Outstanding adsorption per-formance of graphene-carbon nanotube aerogels for continuous oil removal[J]. Carbon, 2014, 80:523-533.
[25] Wan W, Zhang R, Li W, et al. Graphene-carbon nanotube aerogel as an ultra-light,compressible and recyclable highly efficient ab-sorbent for oil and dyes[J]. Environmental Science:Nano, 2016, 3(1):107-113.
[26] 张凯, 闫小强, 唐自清, 等. 高吸油性三聚氰胺泡沫的制备与性能研究[J]. 河南理工大学学报:自然科学版, 2020, 39(4):155-160.
[27] Lv X, Tian D, Peng Y, et al. Superhydrophobic magnetic reduced graphene oxide-decorated foam for efficient and repeatable oil-waterseparation[J]. Applied Surface Science, 2019, 466:937-945.
[28] Meng H, Yan T, Yu J, et al. Super-hydrophobic and super-lipophi-lic functionalized graphene oxide/polyurethane sponge applied for oil/water separation[J]. Chinese Journal of Chemical Engineering, 2018, 26(5):957-963.
[29] Xia C, Li Y, Fei T, et al. Facile one-pot synjournal of superhydropho-bic reduced graphene oxide-coated polyurethane sponge at the pre-sence of ethanol for oil-water separation[J]. Chemical Engineering Journal, 2018, 345:648-658.
[30] Zhou S, Hao G, Zhou X, et al. One-pot synjournal of robust superhy-drophobic,functionalized graphene/polyurethane sponge for effec-tive continuous oil-water separation[J]. Chemical Engineering Jo-urnal, 2016, 302:155-162.
[31] Zhang L, Li H, Lai X, et al. Thiolated graphene-based superhy-drophobic sponges for oil-water separation[J]. Chemical Engineer-ing Journal, 2017, 316:736-743.
[32] Cao Ning, Guo Jingyu, Boukherroub R, et al. Robust superhydropho-bic polyurethane sponge functionalized with perfluorinated grap-hene oxide for efficient immiscible oil/water mixture,stable emul-sion separation and crude oil dehydration[J]. Science China Tech-nological Sciences, 2019, 62(9):1585-1595.
[33] 李华. 复合泡沫结构吸油材料的合成及性能研究[D]. 大连:大连理工大学, 2014.
[34] Junaidi N F D, Othman N H, Fuzil N S, et al. Recent development of graphene oxide-based membranes for oil-water separation:A re-view[J]. Separation and Purification Technology, 2021, 258:1-16.
[35] Asatekin A, Mayes A M. Oil industry wastewater treatment with fouling resistant membranes containing amphiphilic comb copoly-mers[J]. Environmental Science & Technology, 2009, 43(12):4487-4492.
[36] Xue Z, Liu M, Jiang L. Recent developments in polymeric super-oleophobic surfaces[J]. Journal of Polymer Science Part B:Polymer Physics, 2012, 50(17):1209-1224.
[37] 袁静, 廖芳芳, 郭雅妮, 等. 超亲水超疏油油水分离膜的制备及其性能[J]. 化学进展, 2019, 31(1):144-155.
[38] Feng L, Zhang Z, Mai Z, et al. A super-hydrophobic and super-oleo-philic coating mesh film for the separation of oil and water[J]. Angewandte Chemie, 2004, 116(15):2046-2048.
[39] 栗雯绮, 陈文革, 崔晓娟, 等. 氧化石墨烯膜的制备、改性及应用研究进展[J]. 表面技术, 2021, 50(2):199-210.
[40] Zhang X, Zhang Z, Zeng Z, et al. Superoleophobic graphene oxide/halloysite nanotube composite membranes for oil-water separa-tion[J]. Materials Chemistry and Physics, 2021, 263.Doi: 10.1016/j.matchemphys.2021.124347.
[41] Kazemi F, Jafarzadeh Y, Masoumi S, et al. Oil-in-water emulsion separation by PVC membranes embedded with GO-ZnO nanopar-ticles[J]. Journal of Environmental Chemical Engineering, 2021, 9:1-11.
[42] Peng Y, Yu Z, Li F, et al. A novel reduced graphene oxide-based composite membrane prepared via a facile deposition method for multifunctional applications:oil/water separation and cationic dyes removal[J]. Separation and Purification Technology, 2018, 200:130-140.
[43] Abdalla O, Wahab M A, Abdala A. Mixed matrix membranes con-taining aspartic acid functionalized graphene oxide for enhanced oil-water emulsion separation[J]. Journal of Environmental Che-mical Engineering, 2020, 8:1-9.
[44] An Di, Yang Ling, Wang Tingjie, et al. Separation performance of graphene oxide membrane in aqueous solution[J]. Industrial & Engineering Chemistry Research, 2016, 55(17):4803-4810.
[45] Yang S, Sha S, Lu H, et al. Graphene oxide and reduced grapheme oxide coated cotton fabrics with opposite wettability for continuous oil/water separation[J]. Separation and Purification Technology, 2021, 259:1-8.
[46] Dhumal P S, Khose R V, Wadekar P H, et al. Graphene-bentonite supported free-standing,flexible membrane with switchable wetta-bility for selective oil-water separation[J]. Separation and Purifica-tion Technology, 2021, 266:1-28.
[47] Zinadini S, Vatanpour V, Zinatizadeh A A, et al. Preparation and characterization of antifouling graphene oxide/polyethersulfone ul-trafiltration membrane:Application in MBR for dairy wastewater treatment[J]. Journal of Water Process Engineering, 2015, 7:280-294.
[48] Abdel-Karim A, Leaper S, Alberto M, et al. High flux and fouling resistant flat sheet polyethersulfone membranes incorporated with graphene oxide for ultrafiltration applications[J]. Chemical Engi-neering Journal, 2018, 334:789-799.
[49] 王彪, 刘庆旺, 范振忠, 等. 石墨烯衍生物在油水分离中的应用进展[J]. 东北石油大学学报, 2020, 44(4):66-71.
[50] Alammar A, Park S H, Williams C J, et al. Oil-in-water separation with graphene-based nanocomposite membranes for produced water treatment[J]. Journal of Membrane Science, 2020, 603:1-11.
Outlines

/